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Stability and Quenching Correction Accuracy Study of 3H & 14C LiquidScintillation Reference Sources Based on Diisopropylnaphthalene |
XIAO Yang1,ZHANG Hui2,3,MA Yan2,3,LIU Meiling1,LIU Haoran1,LIANG Juncheng1,ZHANG Jinzhao1,4,ZHAO Qing1,FAN Zihao1,ZHANG Han1,LIU Peng4,FAN Fuyou1,DAI Xiongxin2,3 |
1. National Institute of Metrology, Beijing 100029, China
2. China Institute for Radiation Protection, Taiyuan, Shanxi 030006, China
3. Shanxi Provincial Key Laboratory for Translational Nuclear Medicine & Precision Protection, Taiyuan, Shanxi 030006, China
4. Yantai Research Institute, Harbin Engineering University, Yantai, Shandong 264000, China |
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Abstract To establish a quenching correction method for 3H and 14C in aqueous samples with commercial liquid scintillation cocktails, unquenched reference sources and quenched series reference sources of 3H and 14C were prepared with DIN (Diisopropylnaphthalene) scintillation cocktails. The stability of the reference sources was investigated in dark condition at room temperature. The change of the correction efficiency of the quenched series of reference sources was less than 0.5 % after 16 months. The slopes of activity and tSIE of the unquenching reference sources of 3H and 14C were lower than the critical value during 30 months, which meant that these reference sources were stable. The quenching correction accuracy of toluene and DIN quenched series reference sources was compared by correcting 3H and 14C samples consisted of different commercial liquid scintillation cocktails. As a result, the correction curve of DIN reference sources was more suitable for commercial liquid scintillation cocktails such as Ultima GoldTM AB, Ultima GoldTM LLT and Optiphase HiSafe 3.
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Received: 20 December 2023
Published: 29 November 2024
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[1] |
DDEP-Decay Data Evaluation Project [EB/OL]. (2024-02-20).http://www. lnhb.fr/nuclides/H-3_tables.pdf.
|
[8] |
HOU X L, DAI X X. Environmental liquid scintillation analysis [J]. Handbook of Radioactivity Analysis. 2020(2): 41-136.
|
[9] |
姜国华. 液体闪烁测量中的淬灭和淬灭校正 [J]. 中国现代教育装备, 2007(10): 16-21.
|
[20] |
THOMSON J. Dl-ISOPROPYLNAPHTHALENE—A New Solvent for Liquid Scintillation Counting. [J]. Liquid Scintillation Couting and Organic Scintill-Ator, 1987(3): 19-34.
|
[5] |
STOJKOVI I, NIKOLOV J, TOMI M. Biogenic fraction determination in fuels-Optimal parameters survey [J]. Fuel, 2017, 191: 330-338.
|
[3] |
HOU X L. Tritium and 14C in the Environment and Nuclear Facilities: Sources and Analytical Methods [J]. Journal of Nuclear Fuel Cycle and Waste Technology, 2018,16(1):11-39.
|
[4] |
胡崇庆,赵超,刘佳煜. 环境水中氚浓度的液体闪烁计数测量方法及其质量控制 [J]. 计量学报, 2023, 44(11): 1776-1782.
|
[7] |
HOU X L. Rapid analysis of 14C and 3H in graphite and concrete for decommissioning of nuclear reactor [J]. Applied Radiation and Isotopes, 2005, 62(6): 871-882.
|
[10] |
CASSRTTE P, ALTZITZOGLOU T, ANTOHE A, et al. Results of the CCRI(II)-S12.H-3 supplementary comparison: Comparison of methods for the calculation of the activity and standard uncertainty of a tritiated-water source measured using the LSC-TDCR method [J]. Applied Radiation and Isotopes, 2018,134: 257-262.
|
|
WU Y L, LIANG J C, LIU H R,et al. Construction and Implementation of a Liquid Scintillation TDCR System[J].Acta Metrologica Sinica, 2014, 35(1): 83-86.
|
|
WU Y L, LIU H R, LIU J C, et al. Absolute Measurement of Activity of Tritiated Water [J]. Journal of Radioanalytical & Nuclear Chemistry, 2016, 38(1): 32-37.
|
[13] |
TARANCN A, ALONSO E, GARCA J F, et al. Comparative study of quenching correction procedures for 90Sr/90Y determination by Cerenkov, liquid scintillation and plastic scintillation techniques [J]. Analytica Chimica Acta, 2002, 471: 135-143.
|
[2] |
DDEP-Decay Data Evaluation Project [EB/OL]. (2024-02-20).http://www. lnhb.fr/nuclides/C-14_tables.pdf.
|
|
JIANG G H. Quenching and quenching correction in liquid scintillation measurements [J]. Chinese Modern Educational Equipment, 2007(10): 16-21.
|
[14] |
KOSSERT K, XAVIER M. Improved activity standardization of Sr-90/Y-90 by means of liquid scintillation counting [J]. Applied radiation and isotopes, 2020, 168(1): 109478-109484.
|
[16] |
BRODA R, CASSETTE P, KOSSERT K. Radionuclide metrology using liquid scintillation counting [J]. Metrologia, 2007, 44: S36-S52.
|
[17] |
VARLAM C, FAURESCU I, VAGNER I. et al. Nitromethane and other quenching agents used to determine the tritium activity concentration by liquid scintillation spectroscopy [J]. Journal of Radioanalytical and Nuclear Chemistry, 2015, 303: 789-795.
|
|
MA Y, ZHANG H, YANG Y G, et al. Identification of 14C Nuclides in 14C-urea Capsules [J]. Atomic Energy Science and Technology, 2023, 57(11): 2162-2169.
|
[21] |
杨守礼, 刘广大, 马海波,等. 美国Beckman公司和上海原子核所的3H 和14C液闪猝灭校正系列源的比较和评价 [J]. 辐射防护, 1989(5): 329-336.
|
|
HU C Q, ZHAO C, LIU J Y. Measurement Method of Tritium Concentration in Environmental Water Using a Liquid Scintillation Counter and Its Quality Control[J]. Acta Metrologica Sinica, 2023, 44(11): 1776-1782.
|
[6] |
NORTON G A. Direct Analysis of Automotive Fuels for Bioethanol Content Using Radiocarbon Analysis [J]. Radiocarbon, 2009, 51: 995-1003.
|
[11] |
吴永乐,梁珺成,刘浩然,等. 液闪TDCR活度测量装置的研制 [J]. 计量学报, 2014, 35(1): 83-86.
|
[12] |
吴永乐, 刘浩然, 柳加成,等. 氚化水放射性活度的绝对测量 [J]. 核化学与放射化学, 2016, 38(1): 32-37.
|
[18] |
马彦,张辉,杨永刚,等. 尿素[14C]胶囊中14C核素的鉴别 [J]. 原子能科学技术,2023,57(11): 2162-2169.
|
[19] |
LIU H R, ZHOU Q Q, FAN F Y, et al. Activity determination of 231Pa by means of liquid scintillation counting [J]. Applied Radiation and Isotopes, 2020 (155): 108944
|
[15] |
WARWICK P E, CROUDACE I W. Identification and Quantification of Radionuclides in Contaminated Drinking Waters and Pipeline Deposits [J]. Analytical Chemistry, 2013, 85(17): 8166-8172.
|
|
YANG S L, LIU G D, MA H B, et al. Comparison and evaluation of 3H and 14C liquid flash quenching correction series from Beckman Corporation and Shanghai Nuclear Research Institute [J]. Radiation Protection, 1989(5): 329-336.
|
|
|
|